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The SCF iteration in pyscf supports only the integer occupancy, which is governed by the get_occ method. To assign fractional occupancy, you need to at least update get_occ . Other methods may need to be overwritten as well. see the APIs

mf : an instance of SCF class
and the example https://github.com/pyscf/pyscf/blob/master/examples/scf/50-mom-deltaSCF.py

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Answer selected by sunqm
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Converted from issue

This discussion was converted from issue #1827 on January 27, 2025 05:23.